Solvated graphene frameworks as high-performance anodes for lithium-ion batteries

Angew Chem Int Ed Engl. 2015 Apr 27;54(18):5345-50. doi: 10.1002/anie.201500677. Epub 2015 Mar 10.

Abstract

A solvent-exchange approach for the preparation of solvated graphene frameworks as high-performance anode materials for lithium-ion batteries is reported. The mechanically strong graphene frameworks exhibit unique hierarchical solvated porous networks and can be directly used as electrodes with a significantly improved electrochemical performance compared to unsolvated graphene frameworks, including very high reversible capacities, excellent rate capabilities, and superior cycling stabilities.

Keywords: anodes; electrochemistry; graphene; lithium-ion batteries; porous materials.