Novel liquid chromatography-mass spectrometry method for sensitive determination of the mustard allergen Sin a 1 in food

Food Chem. 2015 Sep 15:183:58-63. doi: 10.1016/j.foodchem.2015.02.139. Epub 2015 Mar 12.

Abstract

Mustard is a condiment added to a variety of foodstuffs and a frequent cause of food allergy. A new strategy for the detection of mustard allergen in food products is presented. The methodology is based on liquid chromatography analysis coupled to mass spectrometry. Mustard allergen Sin a 1 was purified from yellow mustard seeds. Sin a 1 was detected with a total of five peptides showing a linear response (lowest LOD was 5ng). Sin a 1 was detected in mustard sauces and salty biscuit (19±3mg/kg) where mustard content is not specified. Sin a 1, used as an internal standard, allowed quantification of this mustard allergen in foods. A novel LC/MS/MS SRM-based method has been developed to detect and quantify the presence of mustard. This method could help to detect mustard allergen Sin a 1 in processed foods and protect mustard-allergic consumers.

Keywords: Allergens; Hidden allergen; LC–MS; Mustard allergy; Quantification; SRM; Sin a 1.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antigens, Plant / analysis*
  • Antigens, Plant / immunology
  • Chromatography, Liquid / methods*
  • Food Analysis / methods*
  • Food Hypersensitivity / immunology
  • Mass Spectrometry / methods*
  • Mustard Plant / chemistry*
  • Mustard Plant / immunology
  • Plant Proteins / analysis*
  • Plant Proteins / immunology

Substances

  • Antigens, Plant
  • Plant Proteins
  • Sin a I protein, Sinapis alba