Predicting the right spacing between protein immobilization sites on self-assembled monolayers to optimize ligand binding

Anal Biochem. 2015 Sep 1:484:133-5. doi: 10.1016/j.ab.2015.05.005. Epub 2015 May 15.

Abstract

Self-assembled monolayers designed to immobilize capture antibodies are usually prepared using a mixture of functional and inactive linkers. Here, using low molar ratios (1:1 to 1:100) of the two linkers resulted in loss of binding capability of the anti-EGFR (epidermal growth factor receptor) antibody nimotuzumab, as assessed by surface plasmon resonance imaging. We then developed a simple theoretical model to predict the optimal surface density of the functional linker, taking into account the antibody size and linker diameter. A high (1:1000) dilution of the functional linker yielded the best results. As an advantage, this approach does not require chemical modification of the protein.

Keywords: Antibody; Nimotuzumab; Protein immobilization; Self-assembled monolayer; Surface plasmon resonance; Theoretical model.

MeSH terms

  • Antibodies, Immobilized / chemistry*
  • Antibodies, Immobilized / immunology
  • Antibodies, Monoclonal, Humanized / chemistry
  • Antibodies, Monoclonal, Humanized / immunology
  • ErbB Receptors / immunology
  • Ligands
  • Models, Molecular
  • Surface Properties

Substances

  • Antibodies, Immobilized
  • Antibodies, Monoclonal, Humanized
  • Ligands
  • nimotuzumab
  • ErbB Receptors