Controlled nitrene transfer from a tyrosinase-like arylnitroso-copper complex

Chem Commun (Camb). 2015 Jun 30;51(56):11206-9. doi: 10.1039/c5cc02806j.

Abstract

The reaction between p-nitrosonitrobenzene and the tetramethylpropylenediamine-copper(i) complex yields a dinuclear complex that is structurally and electronically similar to side-on peroxo species known in Cu/O2 chemistry. The complex reacts with di-tert-butylphenolate via nitrene transfer, as observed through an intermediate and the aminophenol product obtained upon reductive work-up.