Characterization of two glycoside hydrolase family 36 α-galactosidases: novel transglycosylation activity, lead-zinc tolerance, alkaline and multiple pH optima, and low-temperature activity

Food Chem. 2016 Mar 1:194:156-66. doi: 10.1016/j.foodchem.2015.08.015. Epub 2015 Aug 5.

Abstract

Two α-galactosidases, AgaAJB07 from Mesorhizobium and AgaAHJG4 from Streptomyces, were expressed in Escherichia coli. Recombinant AgaAJB07 showed a 2.9-fold and 22.6-fold increase in kcat with a concomitant increase of 2.3-fold and 16.3-fold in Km in the presence of 0.5mM ZnSO4 and 30.0mM Pb(CH3COO)2, respectively. Recombinant AgaAHJG4 showed apparent optimal activity at pH 8.0 in McIlvaine or Tris-HCl buffer and 9.5 in glycine-NaOH or HCl-borax-NaOH buffer, retention of 23.6% and 43.2% activity when assayed at 10 and 20°C, respectively, and a half-life of approximately 2min at 50°C. The activation energies for p-nitrophenyl-α-d-galactopyranoside hydrolysis by AgaAJB07 and AgaAHJG4 were 71.9±0.8 and 48.2±2.0kJmol(-1), respectively. Both AgaAJB07 and AgaAHJG4 exhibited transglycosylation activity, but they required different acceptors and produced different compounds. Furthermore, potential factors for alkaline and multiple pH optima and low-temperature adaptations of AgaAHJG4 were presumed.

Keywords: Lead–zinc tolerance; Low-temperature activity; Transglycosylation; pH optimum; α-Galactosidase.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Galactose
  • Glycosides / chemistry*
  • Hydrolysis
  • Lead
  • Temperature
  • Zinc
  • alpha-Galactosidase / chemistry*

Substances

  • Glycosides
  • Lead
  • alpha-Galactosidase
  • Zinc
  • Galactose