Sulfur-Limonene Polysulfide: A Material Synthesized Entirely from Industrial By-Products and Its Use in Removing Toxic Metals from Water and Soil

Angew Chem Int Ed Engl. 2016 Jan 26;55(5):1714-8. doi: 10.1002/anie.201508708. Epub 2015 Oct 20.

Abstract

A polysulfide material was synthesized by the direct reaction of sulfur and d-limonene, by-products of the petroleum and citrus industries, respectively. The resulting material was processed into functional coatings or molded into solid devices for the removal of palladium and mercury salts from water and soil. The binding of mercury(II) to the sulfur-limonene polysulfide resulted in a color change. These properties motivate application in next-generation environmental remediation and mercury sensing.

Keywords: limonene; polysulfide; sulfur; sustainable materials; waste valorization.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Chromatography, Gel
  • Cyclohexenes / chemistry*
  • Limonene
  • Metals / isolation & purification*
  • Microscopy, Electron, Scanning
  • Soil Pollutants / isolation & purification*
  • Sulfides / chemistry*
  • Sulfur / chemistry*
  • Terpenes / chemistry*
  • Water Pollutants, Chemical / isolation & purification*

Substances

  • Cyclohexenes
  • Metals
  • Soil Pollutants
  • Sulfides
  • Terpenes
  • Water Pollutants, Chemical
  • Sulfur
  • Limonene