A novel acetylcholinesterase inhibitor and calcium channel blocker SCR-1693 improves Aβ25-35-impaired mouse cognitive function

Psychopharmacology (Berl). 2016 Feb;233(4):599-613. doi: 10.1007/s00213-015-4133-5. Epub 2015 Nov 11.

Abstract

Rationale: The mechanism involved in AD is complex, which has prompted to develop compounds that could simultaneously interact with several potential targets. Here, we report a new synthesized compound SCR-1693 which is designed to target both AChE and calcium channels that are potential for AD therapy.

Objectives: We investigated the effects of SCR-1693 on AChE and calcium channels, the effects of neuroprotection and anti-amnesia in icv-Aβ25-35-injected mice, and the potential mechanisms.

Methods: AChE activity assay, intracellular Ca(2+) content and calcium currents measurement, and Aβ25-35-induced cellular death determine were performed for validation of designed targets and neuroprotection of SCR-1693. Mice were orally administrated with SCR-1693 once daily after an Aβ25-35 injection. The Morris water maze and Y-maze test, and hippocampal protein detection were conducted on days 5-10, day 11, and day 8. The pyramidal neuron number, hippocampal AChE activity, and synaptic transmission were measured on day 12.

Results: SCR-1693 acted as a selective, reversible, and noncompetitive inhibitor of AChE, and a nonselective voltage-gated calcium channel blocker. SCR-1693 also inhibited the increase of AChE activity in the mouse hippocampus. SCR-1693 was more effective than donepezil and memantine in preventing Aβ25-35-induced long-term and short-term memory impairment, maintaining the basal transmission of Schaffer collateral-CA1 synapses, and sustaining LTP in mouse hippocampus. SCR-1693 attenuated Aβ25-35-induced death of SH-SY5Y cell and the loss of hippocampal pyramidal neurons, and regulated Aβ25-35-induced signal cascade in neurons.

Conclusions: All these findings indicated that SCR-1693, as a double-target-direction agent, is a considerable candidate for AD therapy.

Keywords: AChE inhibitor; Learning and memory; Neuroprotection; SCR-1693; VGCCs blocker; β-Amyloid.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amyloid beta-Peptides / antagonists & inhibitors
  • Amyloid beta-Peptides / toxicity*
  • Animals
  • CHO Cells
  • Calcium Channel Blockers / pharmacology
  • Calcium Channel Blockers / therapeutic use*
  • Cell Line, Tumor
  • Cholinesterase Inhibitors / pharmacology
  • Cholinesterase Inhibitors / therapeutic use*
  • Cognition / drug effects
  • Cognition / physiology
  • Cognition Disorders / chemically induced*
  • Cognition Disorders / drug therapy*
  • Cognition Disorders / metabolism
  • Cricetinae
  • Cricetulus
  • Dose-Response Relationship, Drug
  • HEK293 Cells
  • Humans
  • Male
  • Maze Learning / drug effects
  • Maze Learning / physiology
  • Mice
  • Mice, Inbred ICR
  • Peptide Fragments / antagonists & inhibitors
  • Peptide Fragments / toxicity*
  • Rats
  • Rats, Wistar
  • Tacrine / analogs & derivatives*
  • Tacrine / pharmacology
  • Tacrine / therapeutic use

Substances

  • Amyloid beta-Peptides
  • Calcium Channel Blockers
  • Cholinesterase Inhibitors
  • Peptide Fragments
  • SCR1693
  • amyloid beta-protein (25-35)
  • Tacrine