Cerdulatinib, a novel dual SYK/JAK kinase inhibitor, has broad anti-tumor activity in both ABC and GCB types of diffuse large B cell lymphoma

Oncotarget. 2015 Dec 22;6(41):43881-96. doi: 10.18632/oncotarget.6316.

Abstract

B-cell receptor (BCR) and JAK/STAT pathways play critical roles in diffuse large B-cell lymphoma (DLBCL). Herein, we investigated the anti-lymphoma activity of cerdulatinib, a novel compound that dually targets SYK and JAK/STAT pathways. On a tissue microarray of 62 primary DLBCL tumors, 58% expressed either phosphorylated SYK or STAT3 or both. SYK and STAT3 are also phosphorylated in a panel of eleven DLBCL cell lines although ABC and GCB subtypes exhibited different JAK/STAT and BCR signaling profiles. In both ABC and GCB cell lines, cerdulatinib induced apoptosis that was associated with caspase-3 and PARP cleavage. The compound also blocked G1/S transition and caused cell cycle arrest, accompanied by inhibition of RB phosphorylation and down-regulation of cyclin E. Phosphorylation of BCR components and STAT3 was sensitive to cerdulatinib in both ABC and GCB cell lines under stimulated conditions. Importantly, JAK/STAT and BCR signaling can be blocked by cerdulatinib in primary GCB and non-GCB DLBCL tumor cells that were accompanied by cell death. Our work provides mechanistic insights into the actions of cerdulatinib, suggesting that the drug has a broad anti-tumor activity in both ABC and GCB DLBCL, at least in part by inhibiting SYK and JAK pathways.

Keywords: JAK-STAT; SYK; cerdulatinib; diffuse large B cell lymphoma; molecularly targeted therapy.

MeSH terms

  • Antineoplastic Agents / pharmacology*
  • Cell Line, Tumor
  • Cell Survival / drug effects
  • Enzyme Inhibitors / pharmacology
  • Flow Cytometry
  • Humans
  • Immunoblotting
  • Immunohistochemistry
  • Intracellular Signaling Peptides and Proteins / metabolism
  • Janus Kinases / metabolism
  • Lymphoma, Large B-Cell, Diffuse / pathology*
  • Protein-Tyrosine Kinases / metabolism
  • Pyrimidines / pharmacology*
  • Signal Transduction / drug effects*
  • Sulfones / pharmacology*
  • Syk Kinase
  • Tissue Array Analysis

Substances

  • 4-(cyclopropylamino)-2-((4-(4-(ethylsulfonyl)piperazin-1-yl)phenyl)amino)pyrimidine-5-carboxamide
  • Antineoplastic Agents
  • Enzyme Inhibitors
  • Intracellular Signaling Peptides and Proteins
  • Pyrimidines
  • Sulfones
  • Protein-Tyrosine Kinases
  • Janus Kinases
  • SYK protein, human
  • Syk Kinase