Crosslinking of peanut allergen Ara h 2 by polyphenol oxidase: digestibility and potential allergenicity assessment

J Sci Food Agric. 2016 Aug;96(10):3567-74. doi: 10.1002/jsfa.7542. Epub 2016 Jan 19.

Abstract

Background: Peanut is one of the eight major food allergens. Its allergen, Ara h 2, can be recognized by over 90% of serum IgE samples from peanut-allergic patients. Therefore, reducing the allergenicity of Ara h 2 is especially important.

Results: In the present study, polyphenol oxidase (PPO), a protein cross-linking reaction catalyst that acts on tyrosine residue, was used to modify Ara h 2. After crosslinking, the microstructure, digestibility, IgG binding capability and IgE binding capability of Ara h 2 were analyzed. Cross-linking decreased the potential allergenicity of Ara h 2 by masking the allergen epitope, while the antigenicity of Ara h 2 changed slightly. After crosslinking, the apparent diameter of Ara h 2 was altered from 300 to 1700 nm or 220 nm, indicating that polymerization could either be inter- or intramolecular. Regarding digestibility, crosslinked Ara h 2 was relatively more easily digested by gastric fluid compared with the untreated Ara h 2, but much more difficult in the intestinal fluid.

Conclusion: The crosslinking reaction catalyzed by PPO, as a non-thermal process, may be beneficial for avoiding food allergy. The reaction could mask allergen epitopes, decreasing the allergenicity of Ara h 2. © 2015 Society of Chemical Industry.

Keywords: Ara h 2; allergenicity; antigenicity; cross-linking; digestibility.

MeSH terms

  • 2S Albumins, Plant / chemistry
  • 2S Albumins, Plant / immunology*
  • 2S Albumins, Plant / metabolism*
  • Allergens / chemistry
  • Allergens / immunology
  • Allergens / metabolism
  • Antigens, Plant / chemistry
  • Antigens, Plant / immunology*
  • Antigens, Plant / metabolism*
  • Arachis / immunology*
  • Arachis / metabolism*
  • Catechol Oxidase / metabolism*
  • Digestion
  • Epitopes
  • Glycoproteins / chemistry
  • Glycoproteins / immunology*
  • Glycoproteins / metabolism*
  • Humans
  • Immunoglobulin E / chemistry
  • Protein Binding
  • Protein Structure, Secondary

Substances

  • 2S Albumins, Plant
  • Allergens
  • Antigens, Plant
  • Ara h 2 allergen, Arachis hypogaea
  • Epitopes
  • Glycoproteins
  • Immunoglobulin E
  • Catechol Oxidase