Determination of marbofloxacin in plasma and synovial fluid by ultrafiltration followed by HPLC-MS/MS

J Pharm Biomed Anal. 2016 May 10:123:31-6. doi: 10.1016/j.jpba.2016.01.061. Epub 2016 Feb 1.

Abstract

A rapid LC-MS/MS method for the determination of marbofloxacin in plasma and synovial fluid is presented in this study. The method uses a rapid sample preparation which only requires an ultrafiltration step with centrifugal filter devices. The optimized procedure allows a minimal need of sample (175 μL), particularly useful for synovial fluid samples which amount is rather limited; it is simple, rapid and easily applicable providing anyhow a satisfactory clean up, demonstrated by post-infusion experiments. On the other hand to maximize the speed of the analysis an ultrafast chromatographic separation has been obtained by selecting a column of 20 mm; the reduced run-time is suitable for processing numerous samples on a daily basis. Linearity was assessed in the range 5-2500 ng mL(-1); ofloxacin was used as internal standard. LOD and LOQ were respectively 1 and 5 ng/mL. The method was successfully applied to a set of samples generated during an experimental veterinary study.

Keywords: Bovine; LC–MS/MS; Marbofloxacin; Plasma; Synovial fluid; Ultrafiltration.

MeSH terms

  • Animals
  • Cattle
  • Chromatography, High Pressure Liquid / methods*
  • Fluoroquinolones / blood*
  • Fluoroquinolones / chemistry*
  • Ofloxacin / chemistry
  • Plasma / chemistry*
  • Synovial Fluid / chemistry*
  • Tandem Mass Spectrometry / methods*
  • Ultrafiltration / methods

Substances

  • Fluoroquinolones
  • marbofloxacin
  • Ofloxacin