Pharmacokinetics, pharmacodynamics, and efficacy of a small-molecule SMN2 splicing modifier in mouse models of spinal muscular atrophy

Hum Mol Genet. 2016 May 15;25(10):1885-1899. doi: 10.1093/hmg/ddw062. Epub 2016 Feb 29.

Abstract

Spinal muscular atrophy (SMA) is caused by the loss or mutation of both copies of the survival motor neuron 1 (SMN1) gene. The related SMN2 gene is retained, but due to alternative splicing of exon 7, produces insufficient levels of the SMN protein. Here, we systematically characterize the pharmacokinetic and pharmacodynamics properties of the SMN splicing modifier SMN-C1. SMN-C1 is a low-molecular weight compound that promotes the inclusion of exon 7 and increases production of SMN protein in human cells and in two transgenic mouse models of SMA. Furthermore, increases in SMN protein levels in peripheral blood mononuclear cells and skin correlate with those in the central nervous system (CNS), indicating that a change of these levels in blood or skin can be used as a non-invasive surrogate to monitor increases of SMN protein levels in the CNS. Consistent with restored SMN function, SMN-C1 treatment increases the levels of spliceosomal and U7 small-nuclear RNAs and corrects RNA processing defects induced by SMN deficiency in the spinal cord of SMNΔ7 SMA mice. A 100% or greater increase in SMN protein in the CNS of SMNΔ7 SMA mice robustly improves the phenotype. Importantly, a ∼50% increase in SMN leads to long-term survival, but the SMA phenotype is only partially corrected, indicating that certain SMA disease manifestations may respond to treatment at lower doses. Overall, we provide important insights for the translation of pre-clinical data to the clinic and further therapeutic development of this series of molecules for SMA treatment.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, N.I.H., Extramural

MeSH terms

  • Alternative Splicing / drug effects
  • Alternative Splicing / genetics
  • Animals
  • Central Nervous System / metabolism
  • Disease Models, Animal
  • Dose-Response Relationship, Drug
  • Exons / genetics
  • Humans
  • Isocoumarins / administration & dosage*
  • Leukocytes, Mononuclear / drug effects
  • Mice
  • Mice, Transgenic
  • Muscular Atrophy, Spinal / blood
  • Muscular Atrophy, Spinal / drug therapy*
  • Muscular Atrophy, Spinal / genetics*
  • Muscular Atrophy, Spinal / pathology
  • Piperazines / administration & dosage*
  • RNA Splicing / drug effects
  • RNA Splicing / genetics
  • Skin / metabolism
  • Small Molecule Libraries / administration & dosage
  • Small Molecule Libraries / pharmacokinetics*
  • Survival of Motor Neuron 2 Protein / blood
  • Survival of Motor Neuron 2 Protein / genetics*

Substances

  • Isocoumarins
  • Piperazines
  • SMN-C1 compound
  • SMN2 protein, mouse
  • Small Molecule Libraries
  • Survival of Motor Neuron 2 Protein