Automated DBS microsampling, microscale automation and microflow LC-MS for therapeutic protein PK

Bioanalysis. 2016 Apr;8(7):649-59. doi: 10.4155/bio-2015-0006. Epub 2016 Mar 15.

Abstract

Aim: Reduce animal usage for discovery-stage PK studies for biologics programs using microsampling-based approaches and microscale LC-MS.

Methods & results: We report the development of an automated DBS-based serial microsampling approach for studying the PK of therapeutic proteins in mice. Automated sample preparation and microflow LC-MS were used to enable assay miniaturization and improve overall assay throughput. Serial sampling of mice was possible over the full 21-day study period with the first six time points over 24 h being collected using automated DBS sample collection. Overall, this approach demonstrated comparable data to a previous study using single mice per time point liquid samples while reducing animal and compound requirements by 14-fold.

Conclusion: Reduction in animals and drug material is enabled by the use of automated serial DBS microsampling for mice studies in discovery-stage studies of protein therapeutics.

Keywords: DBS; LC; MS; PD; PK; automation; microflow; microsampling; sample preparation; therapeutic protein.

MeSH terms

  • Amino Acid Sequence
  • Animals
  • Antibodies, Monoclonal / analysis
  • Antibodies, Monoclonal / pharmacokinetics
  • Automation
  • Blood Specimen Collection
  • Chromatography, High Pressure Liquid
  • Dried Blood Spot Testing
  • Half-Life
  • Male
  • Mice
  • Mice, Inbred C57BL
  • Miniaturization
  • Molecular Sequence Data
  • Proteins / analysis*
  • Proteins / pharmacokinetics
  • Tandem Mass Spectrometry

Substances

  • Antibodies, Monoclonal
  • Proteins