One-pot synthesis of a gold nanoparticle-Vmh2 hydrophobin nanobiocomplex for glucose monitoring

Nanotechnology. 2016 May 13;27(19):195701. doi: 10.1088/0957-4484/27/19/195701. Epub 2016 Mar 29.

Abstract

HydrophobinVmh2 is a small amphiphilic protein, which self-assembles on different surfaces and naturally interacts with glucose. Here, we report on the synthesis of a nanobiocomplex made of polyethylene glycol, Vmh2 and gold nanoparticles by a one-step process and on its ability to recognise glucose in an aqueous solution at 0.3-0.6-1.2 mg ml(-1) concentrations. Even though the Vmh2 proteins are intrinsically bonded to the gold core, effective glucose interaction monitoring was demonstrated by using dynamic light scattering, ultraviolet-visible, polarization-modulated infrared reflection-absorption and x-ray photoelectron spectroscopies. Experimental results highlighted an affinity constant of 7.3 ± 0.3 mg ml(-1) between the nanobiosystem and the sugar, and a detection sensitivity of 0.13 ± 0.06 a.u./mg ml(-1).

Publication types

  • Retracted Publication

MeSH terms

  • Fungal Proteins / chemistry*
  • Glucose
  • Gold / chemistry*
  • Metal Nanoparticles / chemistry*
  • Microscopy, Electron, Transmission
  • Particle Size
  • Polyethylene Glycols / chemistry
  • Spectrum Analysis

Substances

  • Fungal Proteins
  • Polyethylene Glycols
  • Gold
  • Glucose