Chemoselective and Sequential Palladium-Catalyzed Couplings for the Generation of Stilbene Libraries via Immobilized Substrates

ACS Comb Sci. 2016 May 9;18(5):225-9. doi: 10.1021/acscombsci.6b00023. Epub 2016 Apr 18.

Abstract

A versatile palladium-catalyzed tandem synthetic sequence to afford E-stilbenes libraries has been developed. Excellent regio- and stereocontrol have been achieved by means of the sequence of Hiyama and Heck cross-couplings. Undesirable homocoupling byproducts were avoided employing immobilized substrates.

Keywords: Heck coupling; Hiyama coupling; palladium cross-coupling reactions; solid-phase organic synthesis.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Catalysis
  • Palladium / chemistry*
  • Small Molecule Libraries / chemical synthesis*
  • Stilbenes / chemical synthesis*

Substances

  • Small Molecule Libraries
  • Stilbenes
  • Palladium