Polychlorinated dibenzo-p-dioxins/furans (PCDD/Fs) and metals in scots pine (Pinus sylvestris) needles from Eastern and Northern Europe: Spatiotemporal patterns, and potential sources

Chemosphere. 2016 Aug:156:30-36. doi: 10.1016/j.chemosphere.2016.04.111. Epub 2016 May 6.

Abstract

Pine needles were sampled to determine levels of polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs) and metals in Scots pine (Pinus sylvestris) needles at industrial, urban and background sites in Sweden (SW), Czech Republic (CZ) and Slovakia (SK). Spatial and temporal patterns of PCDD/Fs in pine needles were investigated and principal component analysis (PCA) used to determine spatial patterns, potential sources and transport of PCDD/Fs. Levels of PCDD/Fs in pine needles were generally greatest near to industrial sites (Ʃ2,3,7,8-PCDD/Fs (lower bound (LB)): 6 ng kg(-1) - 190 ng kg(-1)) compared to urban and background sites (Ʃ2,3,7,8-PCDD/Fs (LB): 0.90 ng kg(-1) - 20 ng kg(-1)). Using metal contamination in pine needles helped to detect spatial patterns and separate local thermal sources of PCDD/Fs.

Keywords: Atmospheric contamination; Europe; Metal; Pine needle; Polychlorinated dibenzo-p-dioxins/furans.

MeSH terms

  • Cities
  • Czech Republic
  • Dibenzofurans, Polychlorinated / analysis*
  • Environmental Monitoring
  • Environmental Pollutants / analysis*
  • Industry
  • Metals / analysis*
  • Pinus sylvestris*
  • Plant Leaves / chemistry*
  • Polychlorinated Dibenzodioxins / analysis*
  • Slovakia
  • Sweden

Substances

  • Dibenzofurans, Polychlorinated
  • Environmental Pollutants
  • Metals
  • Polychlorinated Dibenzodioxins