Imaging of room-temperature ferromagnetic nano-domains at the surface of a non-magnetic oxide

Nat Commun. 2016 Jun 10:7:11781. doi: 10.1038/ncomms11781.

Abstract

Two-dimensional electron gases at oxide surfaces or interfaces show exotic ordered states of matter, like superconductivity, magnetism or spin-polarized states, and are a promising platform for alternative oxide-based electronics. Here we directly image a dense population of randomly distributed ferromagnetic domains of ∼40 nm typical sizes at room temperature at the oxygen-deficient surface of SrTiO3, a non-magnetic transparent insulator in the bulk. We use laser-based photoemission electron microscopy, an experimental technique that gives selective spin detection of the surface carriers, even in bulk insulators, with a high spatial resolution of 2.6 nm. We furthermore find that the Curie temperature in this system is as high as 900 K. These findings open perspectives for applications in nano-domain magnetism and spintronics using oxide-based devices, for instance through the nano-engineering of oxygen vacancies at surfaces or interfaces of transition-metal oxides.

Publication types

  • Research Support, Non-U.S. Gov't