c-Myc Modulation and Acetylation Is a Key HDAC Inhibitor Target in Cancer

Clin Cancer Res. 2017 May 15;23(10):2542-2555. doi: 10.1158/1078-0432.CCR-15-2388. Epub 2016 Jun 29.

Abstract

Purpose: Histone deacetylase inhibitors (HDACi) are promising anticancer drugs. Although some HDACi have entered the clinic, the mechanism(s) underlying their tumor selectivity are poorly understood.Experimental Design and Results: Using gene expression analysis, we define a core set of six genes commonly regulated in acute myeloid leukemia (AML) blasts and cell lines. MYC, the most prominently modulated, is preferentially altered in leukemia. Upon HDACi treatment, c-Myc is acetylated at lysine 323 and its expression decreases, leading to TRAIL activation and apoptosis. c-Myc binds to the TRAIL promoter on the proximal GC box through SP1 or MIZ1, impairing TRAIL activation. HDACi exposure triggers TRAIL expression, altering c-Myc-TRAIL binding. These events do not occur in normal cells. Excitingly, this inverse correlation between TRAIL and c-Myc is supported by HDACi treatment ex vivo of AML blasts and primary human breast cancer cells. The predictive value of c-Myc to HDACi responsiveness is confirmed in vivo in AML patients undergoing HDACi-based clinical trials.Conclusions: Collectively, our findings identify a key role for c-Myc in TRAIL deregulation and as a biomarker of the anticancer action of HDACi in AML. The potential improved patient stratification could pave the way toward personalized therapies. Clin Cancer Res; 23(10); 2542-55. ©2016 AACR.

MeSH terms

  • Acetylation
  • Cell Line, Tumor
  • Clinical Trials as Topic
  • Gene Expression Regulation, Leukemic / drug effects
  • Histone Deacetylase 1 / antagonists & inhibitors
  • Histone Deacetylase 1 / genetics*
  • Histone Deacetylase Inhibitors / administration & dosage
  • Humans
  • Kruppel-Like Transcription Factors / genetics
  • Neoplasms / drug therapy*
  • Neoplasms / pathology
  • Protein Binding
  • Proto-Oncogene Proteins c-myc / genetics*
  • Signal Transduction / drug effects
  • Sp1 Transcription Factor / genetics
  • TNF-Related Apoptosis-Inducing Ligand / genetics*

Substances

  • Histone Deacetylase Inhibitors
  • Kruppel-Like Transcription Factors
  • MYC protein, human
  • Proto-Oncogene Proteins c-myc
  • Sp1 Transcription Factor
  • SP1 protein, human
  • TNF-Related Apoptosis-Inducing Ligand
  • TNFSF10 protein, human
  • ZBTB17 protein, human
  • HDAC1 protein, human
  • Histone Deacetylase 1