Identification of Targets of the HIF-1 Inhibitor IDF-11774 Using Alkyne-Conjugated Photoaffinity Probes

Bioconjug Chem. 2016 Aug 17;27(8):1911-20. doi: 10.1021/acs.bioconjchem.6b00305. Epub 2016 Jul 18.

Abstract

We developed a hypoxia-inducible factor-1 (HIF-1) inhibitor, IDF-11774, as a clinical candidate for cancer therapy. To understand the mechanism of action of IDF-11774, we attempted to isolate target proteins of IDF-11774 using bioconjugated probes. Multifunctional chemical probes containing sites for click conjugation and photoaffinity labeling were designed and synthesized. After fluorescence and photoaffinity labeling of proteins, two-dimensional electrophoresis (2DE) was performed to isolate specific molecular targets of IDF-11774. Heat shock protein (HSP) 70 was identified as a target protein of IDF-11774. We revealed that IDF-11774 inhibited HSP70 chaperone activity by binding to its allosteric pocket, rather than the ATP-binding site in its nucleotide-binding domain (NBD). Moreover, IDF-11774 reduced the oxygen consumption rate (OCR) and ATP production, thereby increasing intracellular oxygen tension. This result suggests that the inhibition of HSP70 chaperone activity by IDF-11774 suppresses HIF-1α refolding and stimulates HIF-1α degradation. Taken together, these findings indicate that IDF-11774-derived chemical probes successfully identified IDF-11774's target molecule, HSP70, and elucidated the mode of action of IDF-11774 in inhibiting HSP70 chaperone activity and stimulating HIF-1α degradation in cancer cells.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adamantane / analogs & derivatives*
  • Adamantane / pharmacology
  • Adenosine Triphosphate / biosynthesis
  • Alkynes / chemistry*
  • Allosteric Site / drug effects
  • Benzoic Acid / pharmacology*
  • Cell Respiration / drug effects
  • HCT116 Cells
  • HSP70 Heat-Shock Proteins / antagonists & inhibitors*
  • HSP70 Heat-Shock Proteins / chemistry*
  • HSP70 Heat-Shock Proteins / metabolism
  • Humans
  • Hypoxia-Inducible Factor 1 / antagonists & inhibitors*
  • Mitochondria / drug effects
  • Mitochondria / metabolism
  • Models, Molecular
  • Piperazines / pharmacology*
  • Protein Conformation
  • Protein Domains
  • Staining and Labeling

Substances

  • Alkynes
  • HSP70 Heat-Shock Proteins
  • Hypoxia-Inducible Factor 1
  • IDF-11774
  • Piperazines
  • Adenosine Triphosphate
  • Benzoic Acid
  • Adamantane