Nucleic Acid Templated Chemical Reaction in a Live Vertebrate

ACS Cent Sci. 2016 Jun 22;2(6):394-400. doi: 10.1021/acscentsci.6b00054. Epub 2016 May 18.

Abstract

Nucleic acid templated reactions are enabled by the hybridization of probe-reagent conjugates resulting in high effective reagent concentration and fast chemical transformation. We have developed a reaction that harnesses cellular microRNA (miRNA) to yield the cleavage of a linker releasing fluorogenic rhodamine in a live vertebrate. The reaction is based on the catalytic photoreduction of an azide by a ruthenium complex. We showed that this system reports specific expression of miRNA in living tissues of a vertebrate.