ATP-dependent substrate transport by the ABC transporter MsbA is proton-coupled

Nat Commun. 2016 Aug 8:7:12387. doi: 10.1038/ncomms12387.

Abstract

ATP-binding cassette transporters mediate the transbilayer movement of a vast number of substrates in or out of cells in organisms ranging from bacteria to humans. Current alternating access models for ABC exporters including the multidrug and Lipid A transporter MsbA from Escherichia coli suggest a role for nucleotide as the fundamental source of free energy. These models involve cycling between conformations with inward- and outward-facing substrate-binding sites in response to engagement and hydrolysis of ATP at the nucleotide-binding domains. Here we report that MsbA also utilizes another major energy currency in the cell by coupling substrate transport to a transmembrane electrochemical proton gradient. The dependence of ATP-dependent transport on proton coupling, and the stimulation of MsbA-ATPase by the chemical proton gradient highlight the functional integration of both forms of metabolic energy. These findings introduce ion coupling as a new parameter in the mechanism of this homodimeric ABC transporter.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • ATP-Binding Cassette Transporters / chemistry
  • ATP-Binding Cassette Transporters / isolation & purification
  • ATP-Binding Cassette Transporters / metabolism*
  • Adenosine Triphosphate / metabolism*
  • Amino Acid Sequence
  • Bacterial Proteins / chemistry
  • Bacterial Proteins / isolation & purification
  • Bacterial Proteins / metabolism*
  • Biological Transport / drug effects
  • Chloramphenicol / pharmacology
  • Electrochemistry
  • Ethidium / metabolism
  • Hydrolysis
  • Ions
  • Proteolipids / metabolism
  • Protons*
  • Substrate Specificity / drug effects

Substances

  • ATP-Binding Cassette Transporters
  • Bacterial Proteins
  • Ions
  • MsbA protein, Bacteria
  • Proteolipids
  • Protons
  • proteoliposomes
  • Chloramphenicol
  • Adenosine Triphosphate
  • Ethidium