Crystallinity Engineering of Hematite Nanorods for High-Efficiency Photoelectrochemical Water Splitting

Adv Sci (Weinh). 2015 Mar 16;2(4):1500005. doi: 10.1002/advs.201500005. eCollection 2015 Apr.

Abstract

An effective strategy to overcome the morphology evolution of hematite nanorods under high-temperature activation is presented, via tuning the crystallinity and sintering temperature by substrate modification. It is demonstrated that the as-prepared doping-free hematite nanorods with fine nanostructures obtain a significantly higher photocurrent density of 2.12 mA cm-2 at 1.23 V versus RHE, due to effective charge separation and transfer.

Keywords: antimony‐doped tin oxide nanoparticles; conductive substrate modification; crystallinity engineering; hematite nanorod; photoelectrochemical.