MK-8776, a novel chk1 kinase inhibitor, radiosensitizes p53-defective human tumor cells

Oncotarget. 2016 Nov 1;7(44):71660-71672. doi: 10.18632/oncotarget.12311.

Abstract

Radiotherapy is commonly used to treat a variety of solid tumors but improvements in the therapeutic ratio are sorely needed. The aim of this study was to assess the Chk1 kinase inhibitor, MK-8776, for its ability to radiosensitize human tumor cells. Cells derived from NSCLC and HNSCC cancers were tested for radiosensitization by MK-8776. The ability of MK-8776 to abrogate the radiation-induced G2 block was determined using flow cytometry. Effects on repair of radiation-induced DNA double strand breaks (DSBs) were determined on the basis of rad51, γ-H2AX and 53BP1 foci. Clonogenic survival analyses indicated that MK-8776 radiosensitized p53-defective tumor cells but not lines with wild-type p53. Abrogation of the G2 block was evident in both p53-defective cells and p53 wild-type lines indicating no correlation with radiosensitization. However, only p53-defective cells entered mitosis harboring unrepaired DSBs. MK-8776 appeared to inhibit repair of radiation-induced DSBs at early times after irradiation. A comparison of MK-8776 to the wee1 inhibitor, MK-1775, suggested both similarities and differences in their activities. In conclusion, MK-8776 radiosensitizes tumor cells by mechanisms that include abrogation of the G2 block and inhibition of DSB repair. Our findings support the clinical evaluation of MK-8776 in combination with radiation.

Keywords: Chk1; DNA damage; MK-8776; p53-dependent; radiation.

MeSH terms

  • Cell Line, Tumor
  • Checkpoint Kinase 1 / antagonists & inhibitors*
  • DNA Breaks, Double-Stranded
  • G2 Phase / radiation effects
  • Histones / analysis
  • Humans
  • Pyrazoles / pharmacology*
  • Pyrimidines / pharmacology*
  • Pyrimidinones
  • Radiation-Sensitizing Agents / pharmacology*
  • Tumor Suppressor Protein p53 / genetics
  • Tumor Suppressor Protein p53 / physiology*

Substances

  • H2AX protein, human
  • Histones
  • MK-8776
  • Pyrazoles
  • Pyrimidines
  • Pyrimidinones
  • Radiation-Sensitizing Agents
  • TP53 protein, human
  • Tumor Suppressor Protein p53
  • Checkpoint Kinase 1
  • adavosertib