A polyamidoamne dendrimer functionalized graphene oxide for DOX and MMP-9 shRNA plasmid co-delivery

Mater Sci Eng C Mater Biol Appl. 2017 Jan 1;70(Pt 1):572-585. doi: 10.1016/j.msec.2016.09.035. Epub 2016 Sep 19.

Abstract

It is a promising way to treat the multi drug resistance (MDR) of tumor cells in both of drug and gene methods. A polyamidoamne dendrimer functionalized graphene oxide (GO-PAMAM) was designed, which could load doxorubicin (DOX) and MMP-9 shRNA plasmid at the same time in order to achieve effective treatment to breast cancer. GO-PAMAM has a high loading capacity to DOX and pH-controlled DOX release. Besides, it has efficient gene transfer ability, the transfection efficiency is significantly better than PEI-25k in the presence of serum, and it can significantly inhibit the expression of MMP-9 protein in MCF-7 cells. The effect of DOX and MMP-9 shRNA plasmid co-delivery was more significant than that of the single drug. Moreover, GO-PAMAM exhibited lower cytotoxicity compared to PEI-25k in CCK-8 assays, and also showed a good biocompatibility in vivo. Therefore, GO-PAMAM will have broad prospects for drug and gene co-delivery.

Keywords: Co-delivery; DOX; Dendrimer; Graphene oxide; MMP-9 shRNA plasmid.

MeSH terms

  • 3T3 Cells
  • Animals
  • Apoptosis / drug effects
  • Biocompatible Materials / pharmacology
  • Cell Survival / drug effects
  • DNA / metabolism
  • Dendrimers / chemical synthesis
  • Dendrimers / chemistry*
  • Doxorubicin / pharmacology*
  • Drug Delivery Systems*
  • Drug Liberation
  • Electrophoresis, Agar Gel
  • Flow Cytometry
  • Gene Transfer Techniques*
  • Graphite / chemistry*
  • Humans
  • Inhibitory Concentration 50
  • MCF-7 Cells
  • Matrix Metalloproteinase 9 / metabolism
  • Mice
  • Plasmids / administration & dosage*
  • RNA, Small Interfering / administration & dosage*
  • Spectroscopy, Fourier Transform Infrared
  • Spectrum Analysis, Raman
  • Static Electricity
  • Thermogravimetry
  • Transfection

Substances

  • Biocompatible Materials
  • Dendrimers
  • PAMAM Starburst
  • RNA, Small Interfering
  • Graphite
  • Doxorubicin
  • DNA
  • Matrix Metalloproteinase 9