Single-Molecule Imaging With One Color Fluorescence

Methods Enzymol. 2016:581:33-51. doi: 10.1016/bs.mie.2016.08.011. Epub 2016 Oct 7.

Abstract

Single-molecule fluorescence imaging is a powerful tool that enables real-time observation of DNA-protein or RNA-protein interactions with a nanometer precision. Here, we provide a detailed procedure for a previously developed single-molecule fluorescence method, termed "single-molecule protein-induced fluorescence enhancement" (smPIFE). While smFRET (Förster resonance energy transfer) requires both donor and acceptor, protein-induced fluorescence enhancement (PIFE) employs a single dye and measures the increase in fluorescence intensity induced by protein binding near the dye. PIFE displays distance sensitivity within 0-4nm, making it a powerful complementary or alternative tool to FRET method. In this chapter, we will discuss the various ways that PIFE has been utilized to study protein-nucleic acid interactions.

Keywords: Förster resonance energy transfer; One-color imaging; Protein–nucleic acid interactions; Single-molecule protein-induced fluorescence enhancement.

MeSH terms

  • DNA / chemistry
  • DNA / isolation & purification*
  • DNA-Binding Proteins / chemistry
  • DNA-Binding Proteins / isolation & purification*
  • Fluorescence Resonance Energy Transfer
  • Fluorescent Dyes / chemistry
  • Molecular Imaging / methods*
  • Protein Binding
  • RNA-Binding Proteins / chemistry
  • RNA-Binding Proteins / isolation & purification*
  • Spectrometry, Fluorescence / methods

Substances

  • DNA-Binding Proteins
  • Fluorescent Dyes
  • RNA-Binding Proteins
  • DNA