Investigation of the derivatization conditions for GC-MS metabolomics of biological samples

Bioanalysis. 2017 Jan;9(1):53-65. doi: 10.4155/bio-2016-0224.

Abstract

Aim: Metabolomics applications represent an emerging field where significant efforts are directed. Derivatization consists prerequisite for GC-MS metabolomics analysis.

Methods: Common silylation agents were tested for the derivatization of blood plasma. Optimization of methoxyamination and silylation reactions was performed on a mixture of reference standards, consisting of 46 different metabolites. Stability of derivatized metabolites was tested at 4°C.

Results: Optimum results were achieved using N-methyl-N-(trimethylsilyl)trifluoroacetamide. Methoxyamination at room temperature for 24 h followed by 2-h silylation at high temperature lead to efficient derivatization.

Conclusion: Formation and stability of derivatives among metabolites differ greatly, so derivatization should be studied before application in metabolomics studies.

Keywords: GC–MS; derivatization; metabolomics.

MeSH terms

  • Acetamides / chemistry
  • Amination
  • Fluoroacetates / chemistry
  • Gas Chromatography-Mass Spectrometry / methods*
  • Humans
  • Indicators and Reagents
  • Metabolomics / methods*
  • Plasma / chemistry
  • Plasma / metabolism*
  • Trimethylsilyl Compounds / chemistry

Substances

  • Acetamides
  • Fluoroacetates
  • Indicators and Reagents
  • Trimethylsilyl Compounds
  • N-methyl-N-(trimethylsilyl)trifluoroacetamide