The Natural Plant Product Rottlerin Activates Kv7.1/KCNE1 Channels

Cell Physiol Biochem. 2016;40(6):1549-1558. doi: 10.1159/000453205. Epub 2016 Dec 21.

Abstract

Background/aims: Acquired as well as inherited channelopathies are disorders that are caused by altered ion channel function. A family of channels whose malfunction is associated with different channelopathies is the Kv7 K+ channel family; and restoration of normal Kv7 channel function by small molecule modulators is a promising approach for treatment of these often fatal diseases.

Methods: Here, we show the modulation of Kv7 channels by the natural compound Rottlerin heterologously expressed in Xenopus laevis oocytes and on iPSC cardiomyocytes overexpressing Kv7.1 channels.

Results: We show that currents carried by Kv7.1 (EC50 = 1.48 μM), Kv7.1/KCNE1 (EC50 = 4.9 μM), and Kv7.4 (EC50 = 0.148 μM) are strongly enhanced by the compound, whereas Kv7.2, Kv7.2/Kv7.3, and Kv7.5 are not sensitive to Rottlerin. Studies on Kv7.1/KCNE1 mutants and in silico modelling indicate that Rottlerin binds to the R-L3-activator site. Rottlerin mediated activation of Kv7.1/KCNE1 channels might be a promising approach in long QT syndrome. As a proof of concept, we show that Rottlerin shortens cardiac repolarisation in iPSC-derived cardiomyocytes expressing Kv7.1.

Conclusion: Rottlerin or an optimized derivative holds a potential as QT interval correcting drug.

MeSH terms

  • Acetophenones / chemistry
  • Acetophenones / pharmacology*
  • Animals
  • Benzopyrans / chemistry
  • Benzopyrans / pharmacology*
  • Biological Products / chemistry
  • Biological Products / pharmacology*
  • Computer Simulation
  • Humans
  • Induced Pluripotent Stem Cells / cytology
  • Ion Channel Gating / drug effects*
  • KCNQ1 Potassium Channel / chemistry
  • KCNQ1 Potassium Channel / metabolism*
  • Membrane Potentials / drug effects
  • Myocytes, Cardiac / cytology
  • Myocytes, Cardiac / drug effects
  • Myocytes, Cardiac / metabolism
  • Protein Domains
  • Protein Multimerization / drug effects
  • Xenopus laevis

Substances

  • Acetophenones
  • Benzopyrans
  • Biological Products
  • KCNQ1 Potassium Channel
  • rottlerin