Synthesis of Boriranes by Double Hydroboration Reactions of N-Heterocyclic Carbene Boranes and Dimethyl Acetylenedicarboxylate

J Am Chem Soc. 2017 Feb 8;139(5):1726-1729. doi: 10.1021/jacs.6b09873. Epub 2017 Jan 24.

Abstract

Reaction of bis-(2,6-diisopropylphenyl)-imidazol-2-ylidene borane with dimethyl acetylenedicarboxylate gives 80% yield of a stable borirane (boracyclopropane) formed by formal double hydroboration along with 5% of the (E)-alkenylborane. DFT calculations suggest a mechanism where divergence to the two products occurs after a common initial stage of hydride transfer from the NHC-borane to the acetylenedicarboxylate.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.