Quantification of meropenem in human plasma by HILIC - tandem mass spectrometry

J Chromatogr B Analyt Technol Biomed Life Sci. 2017 Mar 1:1046:13-17. doi: 10.1016/j.jchromb.2017.01.016. Epub 2017 Jan 19.

Abstract

Meropenem is a substance from the carbapenem class of antibiotics. It is widely used in intensive care units to treat a broad range of severe bacterial infections. In this critically ill patient group therapeutic drug monitoring (TDM) is highly advisable in order to avoid under- as well as over-dosing. Here, we describe a HILIC-MS/MS method for the quantification of meropenem in human plasma which is suitable for TDM. After simple protein precipitation, the polar analyte was chromatographically separated by the HILIC mechanism on a silica based stationary phase with polyethylenimide coating. The calibration was linear over the range of 1-50μg/ml. The stable isotope labelled internal standard led to matrix independency of the quantification and to very good precision (relative standard deviations less than 5%) and accuracy (deviations from the expected values less than 4%). A cross-validation with a validated and established HPLC-UV method confirmed the accuracy of the HILIC-MS/MS method in real patient samples.

Keywords: Human plasma; Hydrophilic interaction liquid chromatography; Meropenem; Tandem mass spectrometry; Therapeutic drug monitoring.

MeSH terms

  • Chromatography, High Pressure Liquid / methods*
  • Drug Monitoring / methods*
  • Humans
  • Hydrophobic and Hydrophilic Interactions
  • Linear Models
  • Meropenem
  • Reproducibility of Results
  • Sensitivity and Specificity
  • Tandem Mass Spectrometry / methods*
  • Thienamycins / blood*

Substances

  • Thienamycins
  • Meropenem