Both Intrinsic Substrate Preference and Network Context Contribute to Substrate Selection of Classical Tyrosine Phosphatases

J Biol Chem. 2017 Mar 24;292(12):4942-4952. doi: 10.1074/jbc.M116.757518. Epub 2017 Feb 3.

Abstract

Reversible tyrosine phosphorylation is a widespread post-translational modification mechanism underlying cell physiology. Thus, understanding the mechanisms responsible for substrate selection by kinases and phosphatases is central to our ability to model signal transduction at a system level. Classical protein-tyrosine phosphatases can exhibit substrate specificity in vivo by combining intrinsic enzymatic specificity with the network of protein-protein interactions, which positions the enzymes in close proximity to their substrates. Here we use a high throughput approach, based on high density phosphopeptide chips, to determine the in vitro substrate preference of 16 members of the protein-tyrosine phosphatase family. This approach helped identify one residue in the substrate binding pocket of the phosphatase domain that confers specificity for phosphopeptides in a specific sequence context. We also present a Bayesian model that combines intrinsic enzymatic specificity and interaction information in the context of the human protein interaction network to infer new phosphatase substrates at the proteome level.

Keywords: Bayesian integration; peptide array; protein-protein interaction; recognition specificity; substrate specificity; systems biology; trapping mutants; tyrosine-protein phosphatase (tyrosine phosphatase).

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Bayes Theorem
  • Binding Sites
  • Humans
  • Models, Biological
  • Molecular Docking Simulation
  • Phosphopeptides / chemistry
  • Phosphopeptides / metabolism*
  • Phosphorylation
  • Protein Conformation
  • Protein Domains
  • Protein Interaction Maps
  • Protein Tyrosine Phosphatases / chemistry
  • Protein Tyrosine Phosphatases / metabolism*
  • Substrate Specificity

Substances

  • Phosphopeptides
  • Protein Tyrosine Phosphatases