Fast protonation of adenosine and of its radical anion formed by hydrated electron attack; a nanosecond optical and dc-conductivity pulse radiolysis study

Int J Radiat Biol Relat Stud Phys Chem Med. 1987 Nov;52(5):745-53. doi: 10.1080/09553008714552251.

Abstract

The study of the reaction of the hydrated electron with adenosine by optical and dc-conductivity pulse radiolysis on nano- and microsecond timescales has been carried out in an attempt to answer the question whether the electron adduct radical becomes protonated or not. The following conclusions have been reached: (1) the reaction of the hydrated electron with adenosine is followed by a water-mediated protonation, which must be complete with 5 ns; (2) no spectral indication of a further protonation of the protonated electron adduct of adenosine of 2'-deoxyadenosine has been found between 40 and 5000 ns; (3) the equilibrium reaction between radiation produced H3O+ and adenosine with a pKa of 3.5 plays an important role in the kinetics of the conductivity transients.

MeSH terms

  • Adenosine*
  • Anions
  • Deoxyadenosines
  • Electrons
  • Protons
  • Pulse Radiolysis / methods
  • Solutions
  • Time Factors
  • Water

Substances

  • Anions
  • Deoxyadenosines
  • Protons
  • Solutions
  • Water
  • Adenosine