A field-based disparity analysis of new 1,2,5-oxadiazole derivatives endowed with antiproliferative activity

Chem Biol Drug Des. 2017 Nov;90(5):820-839. doi: 10.1111/cbdd.13003. Epub 2017 May 14.

Abstract

A series of 1,2,5-oxadiazoles were synthesized as new potential antiproliferative agents. The in vitro cytotoxic activity evaluation of title compounds through MTT assay revealed that some of them showed significant activity against the HCT-116 cancer cell line. The field-based disparity analysis provided indications about the electrostatic, hydrophobic, and shape features underlying the cytotoxicity, suggesting that increasing the negative electrostatic field on the heterocyclic core of the structure has positive effects on the activity. The structure-activity relationships (SAR) around a particular compound can be explained allowing for a structural rationale for the differences in activity. The SAR provided by this series of compounds can be exploited to carry out further lead optimization.

Keywords: SAR; X-ray; activity cliff; anticancer agents; heteroaryl amide.

MeSH terms

  • Antineoplastic Agents / chemistry*
  • Antineoplastic Agents / pharmacology*
  • Cell Proliferation / drug effects*
  • Colonic Neoplasms / drug therapy
  • Drug Screening Assays, Antitumor
  • HCT116 Cells
  • Humans
  • Models, Molecular
  • Oxadiazoles / chemistry*
  • Oxadiazoles / pharmacology*
  • Structure-Activity Relationship

Substances

  • Antineoplastic Agents
  • Oxadiazoles