Natural alkaloid bouchardatine ameliorates metabolic disorders in high-fat diet-fed mice by stimulating the sirtuin 1/liver kinase B-1/AMPK axis

Br J Pharmacol. 2017 Aug;174(15):2457-2470. doi: 10.1111/bph.13855. Epub 2017 Jun 21.

Abstract

Background and purpose: Promoting energy metabolism is known to provide therapeutic effects for obesity and associated metabolic disorders. The present study evaluated the therapeutic effects of the newly identified bouchardatine (Bou) on obesity-associated metabolic disorders and the molecular mechanisms of these effects.

Experimental approach: The molecular mode of action of Bou for its effects on lipid metabolism was first examined in 3T3-L1 adipocytes and HepG2 cells. This was followed by an evaluation of its metabolic effects in mice fed a high-fat diet for 16 weeks with Bou being administered in the last 5 weeks. Further mechanistic investigations were conducted in pertinent organs of the mice and relevant cell models.

Key results: In 3T3-L1 adipocytes, Bou reduced lipid content and increased sirtuin 1 (SIRT1) activity to facilitate liver kinase B1 (LKB1) activation of AMPK. Chronic administration of Bou (50 mg∙kg-1 every other day) in mice significantly attenuated high-fat diet-induced increases in body weight gain, dyslipidaemia and fatty liver without affecting food intake and no adverse effects were detected. These metabolic effects were associated with activation of the SIRT1-LKB1-AMPK signalling pathway in adipose tissue and liver. Of particular note, UCP1 expression and mitochondrial biogenesis were increased in both white and brown adipose tissues of Bou-treated mice. Incubation with Bou induced similar changes in primary brown adipocytes isolated from mice.

Conclusions and implications: Bou may have therapeutic potential for obesity-related metabolic diseases by increasing the capacity of energy expenditure in adipose tissues and liver through a mechanism involving the SIRT1-LKB1-AMPK axis.

MeSH terms

  • 3T3-L1 Cells
  • AMP-Activated Protein Kinases / metabolism*
  • Animals
  • Biological Products / administration & dosage
  • Biological Products / pharmacology*
  • Diet, High-Fat
  • Dose-Response Relationship, Drug
  • Hep G2 Cells
  • Humans
  • Indole Alkaloids / administration & dosage
  • Indole Alkaloids / pharmacology*
  • Liver / drug effects
  • Liver / enzymology
  • Male
  • Metabolic Diseases / chemically induced
  • Metabolic Diseases / drug therapy*
  • Metabolic Diseases / metabolism
  • Mice
  • Mice, Inbred C57BL
  • Molecular Structure
  • Protein Serine-Threonine Kinases / metabolism*
  • Sirtuin 1 / metabolism*
  • Structure-Activity Relationship

Substances

  • Biological Products
  • Indole Alkaloids
  • bouchardatine
  • Protein Serine-Threonine Kinases
  • Stk11 protein, mouse
  • AMP-Activated Protein Kinases
  • Sirt1 protein, mouse
  • Sirtuin 1