Determination of piperidinium ionic liquid cations in environmental water samples by solid phase extraction and hydrophilic interaction liquid chromatography

J Chromatogr A. 2018 Jul 20:1559:136-140. doi: 10.1016/j.chroma.2017.05.015. Epub 2017 May 8.

Abstract

This paper presents a novel analytical method for the determination of piperidinium ionic liquid cations in environmental water by hydrophilic interaction liquid chromatography and solid-phase extraction technology. The left standing, centrifuged and filtered river water samples were first purified and concentrated through the C18 solid phase extraction column, and eluted with 0.02mol/L hydrochloric acid prepared in methanol and deionized water (80/20, v/v). Then the eluents were analyzed by a hydrophilic column combined with 0.8mmol/L 1-propyl-3-methyl imidazolium tetrafluoroborate aqueous solution/acetonitrile (40/60, v/v) as the mobile phase and indirect ultraviolet detection. The detection limits of piperidinium cations were less than 0.4mg/L. The relative standard deviations were less than 0.6%. The method has been successfully applied to the determination of piperidinium cations in Songhua River water samples. Recoveries were 80.0%-98.3%. This research may provide a reference for studying the environmental effect of ionic liquids.

Keywords: Hydrophilic interaction liquid chromatography; Indirect ultraviolet detection; Ionic liquids; Piperidinium cations; Solid phase extraction.

MeSH terms

  • Cations / chemistry
  • Chromatography, High Pressure Liquid
  • Hydrophobic and Hydrophilic Interactions
  • Ionic Liquids / analysis*
  • Ionic Liquids / isolation & purification
  • Limit of Detection
  • Piperidines / chemistry*
  • Rivers / chemistry
  • Solid Phase Extraction
  • Water Pollutants, Chemical / analysis*
  • Water Pollutants, Chemical / isolation & purification

Substances

  • Cations
  • Ionic Liquids
  • Piperidines
  • Water Pollutants, Chemical