Conformationally restricted analogs of somatostatin with high mu-opiate receptor specificity

Proc Natl Acad Sci U S A. 1985 Jan;82(1):236-9. doi: 10.1073/pnas.82.1.236.

Abstract

A series of cyclic, conformationally restricted analogs of somatostatin have been prepared and tested for their ability to inhibit the binding of [3H]naloxone and [D-Ala2, D-Leu5] [3H]enkephalin to rat brain membranes. The most potent analog, D-Phe-Cys-Tyr-D-Trp-Lys-Thr-Pen-Thr-NH2 where Pen is penicillamine in [D-Phe5, Cys6, Tyr7, D-Trp8, Pen11]somatostatin-(5-12)-octapeptide amide, exhibited high affinity for mu-opiate receptors (IC50 value of [3H]naloxone = 3.5 nM), being 7800 times more potent than somatostatin. The cyclic octapeptide also displayed high mu-opiate receptor selectivity with an IC50 [( D-Ala2,D-Leu5]enkephalin)/IC50 (naloxone) ratio of 271. The high affinity and selectivity of the somatostatin analog for mu-opiate receptors may be of use in examining the physiological role(s) of the mu-opiate receptor.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Animals
  • Binding, Competitive
  • Brain / metabolism*
  • Enkephalin, Leucine / analogs & derivatives
  • Enkephalin, Leucine / metabolism
  • Enkephalin, Leucine-2-Alanine
  • Hormones
  • Naloxone / metabolism
  • Protein Conformation
  • Rats
  • Receptors, Opioid / metabolism*
  • Receptors, Opioid, mu
  • Somatostatin / analogs & derivatives*
  • Somatostatin / metabolism
  • Structure-Activity Relationship
  • Synaptosomes / metabolism

Substances

  • Hormones
  • Receptors, Opioid
  • Receptors, Opioid, mu
  • Naloxone
  • Somatostatin
  • Enkephalin, Leucine
  • Enkephalin, Leucine-2-Alanine