Structural characterization and inhibition on α-glucosidase activity of acidic polysaccharide from Annona squamosa

Carbohydr Polym. 2017 Oct 15:174:1-12. doi: 10.1016/j.carbpol.2017.05.092. Epub 2017 Jun 15.

Abstract

The crude polysaccharide (TASP3) was extracted from the fruit pulp of Annona squamosa and then isolated and purified by the combination of grading-alcoholic precipitation and Sephadex G-200. The structure of purified polysaccharide (GASP3-3-I) was determined based on the physicochemical and instrumental analyses. The results indicated that GASP3-3-I was an acidic heteropolysaccharide and its average molecular weight was 2.28×106Da. The monosaccharide composition was analysed by GC-MS and ion chromatography, respectively. It was revealed that GASP3-3-I was consisted of rhamnose, arabinose, xylose, mannose, glucose, galactose, glucuronic acid and galacturonic acid with a molar ratio of 5.06:45.5:5.26:0.63:6.09:31.76:0.49:5.19. Moreover, periodate oxidation reaction, Smith degrading reaction, methylation, FT-IR and NMR were used to conduct the structural characterization of GASP3-3-I. The results indicated that glycosyl residues of GASP3-3-I were mainly composed of (1→) l-arabinose, (1→6), (1→3) and (1,3→6) d-galactose, (1→) d-xylose, (3→) and (3→6) d-glucose, (1→2) l-rhamnose. The α-glucosidase inhibitory activity assay showed that GASP3-3-I had a certain inhibition on α-glucosidase activity.

Keywords: Acidic polysaccharide; Annona squamosa; Characterization; Structure.

MeSH terms

  • Annona / chemistry*
  • Annona / enzymology*
  • Enzyme Activation / drug effects
  • Enzyme Inhibitors / chemistry
  • Enzyme Inhibitors / pharmacology
  • Glycoside Hydrolase Inhibitors / chemistry
  • Glycoside Hydrolase Inhibitors / pharmacology
  • Polysaccharides / chemistry*
  • Polysaccharides / pharmacology*
  • Spectroscopy, Fourier Transform Infrared
  • alpha-Glucosidases / metabolism*

Substances

  • Enzyme Inhibitors
  • Glycoside Hydrolase Inhibitors
  • Polysaccharides
  • alpha-Glucosidases