Ligand activation induces different conformational changes in CXCR3 receptor isoforms as evidenced by plasmon waveguide resonance (PWR)

Sci Rep. 2017 Sep 6;7(1):10703. doi: 10.1038/s41598-017-11151-x.

Abstract

The chemokine receptor CXCR3 plays important roles in angiogenesis, inflammation and cancer. Activation studies and biological functions of CXCR3 are complex due to the presence of spliced isoforms. CXCR3-A is known as a pro-tumor receptor whereas CXCR3-B exhibits anti-tumor properties. Here, we focused on the conformational change of CXCR3-A and CXCR3-B after agonist or antagonist binding using Plasmon Waveguide Resonance (PWR). Agonist stimulation induced an anisotropic response with very distinct conformational changes for the two isoforms. The CXCR3 agonist bound CXCR3-A with higher affinity than CXCR3-B. Using various concentrations of SCH546738, a CXCR3 specific inhibitor, we demonstrated that low SCH546738 concentrations (≤1 nM) efficiently inhibited CXCR3-A but not CXCR3-B's conformational change and activation. This was confirmed by both, biophysical and biological methods. Taken together, our study demonstrates differences in the behavior of CXCR3-A and CXCR3-B upon ligand activation and antagonist inhibition which may be of relevance for further studies aimed at specifically inhibiting the CXCR3A isoform.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Calcium / metabolism
  • Cell Line
  • Drug Discovery
  • Gene Expression
  • Humans
  • Ligands
  • Protein Binding
  • Protein Conformation* / drug effects
  • Protein Isoforms
  • Quantitative Structure-Activity Relationship
  • Receptors, CXCR3 / chemistry*
  • Receptors, CXCR3 / genetics
  • Receptors, CXCR3 / metabolism
  • Signal Transduction

Substances

  • Ligands
  • Protein Isoforms
  • Receptors, CXCR3
  • Calcium