Folding DNA into a Lipid-Conjugated Nanobarrel for Controlled Reconstitution of Membrane Proteins

Angew Chem Int Ed Engl. 2018 Feb 19;57(8):2072-2076. doi: 10.1002/anie.201710147. Epub 2018 Jan 9.

Abstract

Building upon DNA origami technology, we introduce a method to reconstitute a single membrane protein into a self-assembled DNA nanobarrel that scaffolds a nanodisc-like lipid environment. Compared with the membrane-scaffolding-protein nanodisc technique, our approach gives rise to defined stoichiometry, controlled sizes, as well as enhanced stability and homogeneity in membrane protein reconstitution. We further demonstrate potential applications of the DNA nanobarrels in the structural analysis of membrane proteins.

Keywords: DNA nanotechnology; DNA origami; cryo-EM; membrane protein reconstitution; single-particle analysis.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Cryoelectron Microscopy
  • DNA / chemistry*
  • Glucosides / chemistry
  • Hemolysin Proteins / chemistry
  • Hemolysin Proteins / metabolism
  • Lipids / chemistry*
  • Membrane Proteins / chemistry*
  • Membrane Proteins / metabolism
  • Microscopy, Electron, Transmission
  • Nanostructures / chemistry*

Substances

  • Glucosides
  • Hemolysin Proteins
  • Lipids
  • Membrane Proteins
  • octyl-beta-D-glucoside
  • DNA