Dual-Targeted Selenium Nanoparticles for Synergistic Photothermal Therapy and Chemotherapy of Tumors

Chem Asian J. 2018 Apr 16;13(8):996-1004. doi: 10.1002/asia.201800048. Epub 2018 Mar 13.

Abstract

A combination of chemo- and photothermal therapy has emerged as a promising tactic for cancer therapy. However, the intricacy of accurate delivery and the ability to initiate drug release in specific tumor sites remains a challenging puzzle. Hence, to assure that the chemotherapeutic drug and photothermal agent are synchronously delivered to a tumor area for their synergistic effect, dual-target (RC-12 and PG-6 peptides) functionalized selenium nanoparticles loaded with both doxorubicin (DOX) and indocyanine green (ICG) were designed and successfully synthesized. The as-synthesized nanoparticles exhibited good monodispersity, size stability, and consistent spectral characteristics compared with those of ICG or DOX alone. The nanoparticles underwent self-immolated cleavage under irradiation from a near-IR laser and released the loaded drug owing to sufficient hyperthermia. Moreover, the internalized nanoparticles triggered the overproduction of intracellular reactive oxygen species to induce cell apoptosis. Taken together, this study provides a sequentially triggered nanosystem to achieve precise drug delivery by chemo-photothermal combination.

Keywords: cancer; drug delivery; nanoparticles; photochemistry; selenium.

MeSH terms

  • Apoptosis / drug effects
  • Cell Movement / drug effects
  • Cell-Penetrating Peptides / chemical synthesis
  • Cell-Penetrating Peptides / radiation effects
  • Cell-Penetrating Peptides / therapeutic use*
  • Doxorubicin / chemistry
  • Doxorubicin / pharmacology*
  • Drug Carriers / chemical synthesis
  • Drug Carriers / radiation effects
  • Drug Carriers / therapeutic use*
  • Drug Design
  • Heating
  • Hep G2 Cells
  • Humans
  • Indocyanine Green / chemistry
  • Indocyanine Green / pharmacology*
  • Light
  • Nanoparticles / chemistry
  • Nanoparticles / radiation effects
  • Nanoparticles / therapeutic use*
  • Particle Size
  • Photochemotherapy / methods
  • Reactive Oxygen Species / metabolism

Substances

  • Cell-Penetrating Peptides
  • Drug Carriers
  • Reactive Oxygen Species
  • Doxorubicin
  • Indocyanine Green