Predicting ligand binding poses for low-resolution membrane protein models: Perspectives from multiscale simulations

Biochem Biophys Res Commun. 2018 Mar 29;498(2):366-374. doi: 10.1016/j.bbrc.2018.01.160. Epub 2018 Feb 2.

Abstract

Membrane receptors constitute major targets for pharmaceutical intervention. Drug design efforts rely on the identification of ligand binding poses. However, the limited experimental structural information available may make this extremely challenging, especially when only low-resolution homology models are accessible. In these cases, the predictions may be improved by molecular dynamics simulation approaches. Here we review recent developments of multiscale, hybrid molecular mechanics/coarse-grained (MM/CG) methods applied to membrane proteins. In particular, we focus on our in-house MM/CG approach. It is especially tailored for G-protein coupled receptors, the largest membrane receptor family in humans. We show that our MM/CG approach is able to capture the atomistic details of the receptor/ligand binding interactions, while keeping the computational cost low by representing the protein frame and the membrane environment in a highly simplified manner. We close this review by discussing ongoing improvements and challenges of the current implementation of our MM/CG code.

Keywords: Bitter taste receptor; Chemosensory receptor; G-protein coupled receptor; Homology modeling; Molecular docking; Molecular mechanics/coarse-grained simulations.

Publication types

  • Research Support, Non-U.S. Gov't
  • Review

MeSH terms

  • Binding Sites
  • Humans
  • Ligands
  • Membrane Proteins / chemistry*
  • Membrane Proteins / metabolism*
  • Models, Molecular
  • Molecular Dynamics Simulation
  • Receptors, G-Protein-Coupled / chemistry
  • Receptors, G-Protein-Coupled / metabolism

Substances

  • Ligands
  • Membrane Proteins
  • Receptors, G-Protein-Coupled