RbFe(HAsO4)2 and TlFe(HAsO4)2, two new hydrogenarsenates adopting two closely related structure types

Acta Crystallogr E Crystallogr Commun. 2018 May 1;74(Pt 6):766-771. doi: 10.1107/S2056989018006473. eCollection 2018 Jun 1.

Abstract

Rubidium iron bis-[hydrogen arsenate(V)], RbFe(HAsO4)2, and thallium iron bis-[hydrogen arsenate(V)], TlFe(HAsO4)2, were grown under mild hydro-thermal conditions (T = 493 K, 7 d). RbFe(HAsO4)2 adopts the RbFe(HPO4)2 structure type (space group Rc), while TlFe(HAsO4)2 crystallizes in the (NH4)Fe(HPO4)2 structure type (space group P ). Both compounds have tetra-hedral-octa-hedral framework topologies. The M+ cations are located in channels of the respective framework and are disordered in TlFe(HAsO4)2, which may suggest that the M+ cations can move in the channels.

Keywords: RbFe(HAsO4)2; TlFe(HAsO4)2; arsenate; cation disorder; crystal structure; framework structure; hydrogenarsenate(V).

Grants and funding

This work was funded by Doc fForte Fellowship of the Austrian Academy of Sciences to K. Schwendtner grant .