Rotational spectrum of methoxyamine up to 480 GHz: a laboratory study and astronomical search

Astron Astrophys. 2018 Jan:609:A24. doi: 10.1051/0004-6361/201730744. Epub 2017 Dec 22.

Abstract

Aims: Methoxyamine is a potential interstellar amine that has been predicted by gas-grain chemical models for the formation of complex molecules. The aim of this work is to provide direct experimental frequencies of its ground-vibrational state in the millimeter- and submillimeter-wave regions to achieve its detection in the interstellar medium.

Methods: Methoxyamine was chemically liberated from its hydrochloride salt, and its rotational spectrum was recorded at room temperature from 75 to 480 GHz using the millimeter-wave spectrometer in Valladolid. Many observed transitions revealed A-E splitting caused by the internal rotation of the methyl group, which had to be treated with specific internal rotation codes.

Results: Over 400 lines were newly assigned for the most stable conformer of methoxyamine, and a precise set of spectroscopic constants was obtained. Spectral features of methoxyamine were then searched for in the Orion KL, Sgr B2, B1-b, and TMC-1 molecular clouds. Upper limits to the column density of methoxyamine were derived.

Keywords: ISM: individual objects: Orion KL, Sgr B2, B-1b, TMC-1; ISM: molecules; astrochemistry; astronomical databases: miscellaneous; line: identification.