Fractionation of copper activation products in debris samples from the National Ignition Facility

Appl Radiat Isot. 2019 Jan:143:163-175. doi: 10.1016/j.apradiso.2018.10.014. Epub 2018 Oct 23.

Abstract

Nuclear fusion experiments performed at the National Ignition Facility produce radioactive debris, arising in reactions of fast neutrons with the target assembly. We have found that postshot debris collections are fractionated, such that isotope ratios in an individual debris sample may not be representative of the radionuclide inventory produced by the experiment. We discuss the potential sources of this fractionation and apply isotope-correlation techniques to calculate unfractionated isotope ratios that are used in measurements of nuclear reaction cross sections.

Keywords: Fractionated debris; High energy neutrons; National Ignition Facility; Neutron reaction cross sections; Radiochemical diagnostics.