The role of roughage provision on the absorption and disposition of the mycotoxin deoxynivalenol and its acetylated derivatives in calves: from field observations to toxicokinetics

Arch Toxicol. 2019 Feb;93(2):293-310. doi: 10.1007/s00204-018-2368-8. Epub 2018 Dec 10.

Abstract

A clinical case in Belgium demonstrated that feeding a feed concentrate containing considerable levels of deoxynivalenol (DON, 1.13 mg/kg feed) induced severe liver failure in 2- to 3-month-old beef calves. Symptoms disappeared by replacing the highly contaminated corn and by stimulating ruminal development via roughage administration. A multi-mycotoxin contamination was demonstrated in feed samples collected at 15 different veal farms in Belgium. DON was most prevalent, contaminating 80% of the roughage samples (mixed straw and maize silage; average concentration in positives: 637 ± 621 µg/kg, max. 1818 µg/kg), and all feed concentrate samples (411 ± 156 µg/kg, max. 693 µg/kg). In order to evaluate the impact of roughage provision and its associated ruminal development on the gastro-intestinal absorption and biodegradation of DON and its acetylated derivatives (3- and 15-ADON) in calves, a toxicokinetic study was performed with two ruminating and two non-ruminating male calves. Animals received in succession a bolus of DON (120 µg/kg bodyweight (BW)), 15-ADON (50 µg/kg BW), and 3-ADON (25 µg/kg) by intravenous (IV) injection or per os (PO) in a cross-over design. The absolute oral bioavailability of DON was much higher in non-ruminating calves (50.7 ± 33.0%) compared to ruminating calves (4.1 ± 4.5%). Immediately following exposure, 3- and 15-ADON were hydrolysed to DON in ruminating calves. DON and its acetylated metabolites were mainly metabolized to DON-3-glucuronide, however, also small amounts of DON-15-glucuronide were detected in urine. DON degradation to deepoxy-DON (DOM-1) was only observed to a relevant extent in ruminating calves. Consequently, toxicity of DON in calves is closely related to roughage provision and the associated stage of ruminal development.

Keywords: 3- and 15-Acetyldeoxynivalenol; Biodegradation; Calf; Deoxynivalenol; Mycotoxin; Toxicokinetics.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acetylation
  • Animal Feed / analysis*
  • Animal Feed / toxicity
  • Animals
  • Biological Availability
  • Cattle
  • Dietary Exposure / adverse effects
  • Dietary Exposure / analysis
  • Dietary Fiber / analysis
  • Dietary Fiber / pharmacology*
  • Jaundice / chemically induced
  • Jaundice / veterinary
  • Liver / drug effects
  • Liver / enzymology
  • Liver / pathology
  • Liver Failure / chemically induced
  • Liver Failure / pathology
  • Liver Failure / veterinary*
  • Male
  • Rumination, Digestive
  • Trichothecenes / analysis
  • Trichothecenes / pharmacokinetics*
  • Trichothecenes / poisoning
  • Trichothecenes / toxicity*

Substances

  • Dietary Fiber
  • Trichothecenes
  • deoxynivalenol