An improved ultra-high-performance liquid chromatography-tandem mass spectrometric method for the quantitation of dexmedetomidine in small volume of pediatric plasma

Biomed Chromatogr. 2019 Jun;33(6):e4487. doi: 10.1002/bmc.4487. Epub 2019 Feb 7.

Abstract

Dexmedetomidine (Dex), a highly selective α2 -adrenergic agonist, is used primarily for the sedation and anxiolysis of adults and children in the intensive care setting. A sensitive and selective assay for Dex in pediatric plasma was developed by employing ultra-high-performance liquid chromatography-tandem mass spectrometry with d4-Dex as an internal standard. Dex was extracted from 0.1 mL of plasma by micro-elution solid-phase extraction. Separation was achieved with a Waters XBridge C18 column with a flow rate of 0.3 mL/min using a mobile phase comprising 5 mm ammonium acetate buffer with 0.03% formic acid in water and methanol-acetonitrile (50:50, v/v). The intra-day precision (coefficient of variation) and accuracy for quality control samples ranged from 1.32 to 8.91% and from 92.8 to 108%, respectively. The inter-day precision and accuracy ranged from 2.13 to 8.45% and from 97.0 to 104%, respectively. The analytical method showed excellent sensitivity using a small sample volume (0.1 mL) with a lower limit of quantitation of 5 pg/mL. This method is robust and has been successfully employed in a pharmacokinetic study of Dex in neonates and infants postoperative from cardiac surgery.

Keywords: UHPLC-MS/MS; dexmedetomidine; micro-elution solid-phase extraction; pediatrics; pharmacokinetics.

Publication types

  • Clinical Trial, Phase I

MeSH terms

  • Analgesics, Non-Narcotic / blood*
  • Analgesics, Non-Narcotic / chemistry
  • Analgesics, Non-Narcotic / pharmacokinetics
  • Chromatography, High Pressure Liquid / methods*
  • Dexmedetomidine / blood*
  • Dexmedetomidine / chemistry
  • Dexmedetomidine / pharmacokinetics
  • Humans
  • Infant
  • Infant, Newborn
  • Limit of Detection
  • Reproducibility of Results
  • Solid Phase Microextraction / methods*
  • Tandem Mass Spectrometry / methods*

Substances

  • Analgesics, Non-Narcotic
  • Dexmedetomidine