Boosting photocatalytic H2 evolution on g-C3N4 by modifying covalent organic frameworks (COFs)

Chem Commun (Camb). 2019 May 16;55(41):5829-5832. doi: 10.1039/c9cc02144b.

Abstract

Modifying g-C3N4 with covalent organic frameworks (COFs) through imine linkage results in a dramatically enhanced visible-light-driven photocatalytic hydrogen evolution, which reached 10.1 mmol g-1 h-1 when 2 wt% Pt and triethanolamine were used as co-catalyst and sacrificial agent, respectively, corresponding to an apparent quantum efficiency (AQE) of 20.7% at 425 nm.