Differential suppression of delayed-rectifier and inwardly rectifier K+ currents by a group of ent-kaurane-type diterpenoids from Croton tonkinensis, in microglial cells

Eur J Pharmacol. 2019 Aug 5:856:172414. doi: 10.1016/j.ejphar.2019.172414. Epub 2019 May 24.

Abstract

Croton is an extensive flowering plant genus in the spurge family, Euphorbiaceae. Three croton compounds with the common ent-kaurane skeleton were purified from Croton tonkinensis. By using patch-clamp recording technique, we thoroughly examined the effect of a group of croton compounds, croton-01 (ent-18-acetoxy-7α-hydroxykaur-16-en-15-one), croton-02 (ent-7α,14β-dihydroxykaur-16-en-15-one), and croton-03 (ent-1β-acetoxy-7α,14β-dihydroxykaur-16-en-15-one), on the membrane current in SM826 and BV2 microglial cells. Although neither voltage-gated Na+ nor Ca2+ currents were present in these cells, both delayed-rectifier K+ outward (IK(DR)) and inwardly rectifying K+ currents (IK(IR)) were readily detected. Croton-03 differentially caused inhibition of IK(DR) or IK(IR) in a concentration-dependent manner. According to a minimal scheme, the shortening of the time constant in either the IK(DR)-related block or IK(IR) caused by different concentrations of croton-03 was quantitatively estimated with a dissociation constant of 6.45 and 29.5 μM, respectively. In SM826 cells differentiated with β-amyloid, inhibitory action on these K+ currents remained unaltered. In ultraviolet C-irradiated cells, the magnitude of IK(IR) was still decreased by addition of croton-03. Therefore, our study suggests that these ent-kaurane diterpenoids ought to somehow act on the cellular mechanisms by which they influence the functional activities of microglial cells.

Keywords: Croton; Delayed-rectifier K(+) current; Inwardly rectifier K(+) current; Microglial cell; Open-channel kinetics.

MeSH terms

  • Cell Line
  • Croton / chemistry*
  • Delayed Rectifier Potassium Channels / antagonists & inhibitors
  • Delayed Rectifier Potassium Channels / metabolism*
  • Diterpenes, Kaurane / pharmacology*
  • Dose-Response Relationship, Drug
  • Electrophysiological Phenomena / drug effects*
  • Humans
  • Kinetics
  • Microglia / cytology
  • Microglia / drug effects*
  • Microglia / metabolism
  • Plant Leaves / chemistry
  • Potassium / metabolism*
  • Potassium Channel Blockers / pharmacology*
  • Time Factors

Substances

  • Delayed Rectifier Potassium Channels
  • Diterpenes, Kaurane
  • Potassium Channel Blockers
  • Potassium