Perfluorodecanoic acid-induced oxidative stress and DNA damage investigated at the cellular and molecular levels

Ecotoxicol Environ Saf. 2019 Dec 15:185:109699. doi: 10.1016/j.ecoenv.2019.109699. Epub 2019 Sep 24.

Abstract

Perfluorodecanoic acid (PFDA) has been widely used in production of many daily necessities because of its special nature. Althoughtoxic effects of PFDA to organisms have been reported, there is little research on the genotoxicity induced by oxidative stress of PFDA on the cellular and molecular levels simultaneously. Thus, we investigated the DNA oxidative damage caused by PFDA in mouse hepatocytes. On the cellular level, an increase in ROS content indicated that PFDA caused oxidative stress in mouse hepatocytes. In addition, after PFDA exposure, the comet assay confirmed DNA strand breaks and an increased 8-OHdG content demonstrated DNA oxidative damage. On the molecular level, the microenvironment of aromatic amino acids, skeleton and secondary structure of catalase (CAT) were varied after PFDA exposure and the enzyme activity was reduced because PFDA bound near the heme groups of CAT. Moreover, PFDA was shown to interact with DNA molecule by groove binding. This study suggests that PFDA can cause genotoxicity by inducing oxidative stress both on the cellular and molecular levels.

Keywords: Catalase; DNA; Multi-spectra; Oxidative damage; Perfluorodecanoic acid.

MeSH terms

  • Animals
  • Binding Sites
  • Catalase / chemistry
  • Catalase / metabolism
  • Cells, Cultured
  • Comet Assay
  • DNA / chemistry
  • DNA Damage*
  • Decanoic Acids / toxicity*
  • Environmental Pollutants / toxicity*
  • Fluorocarbons / toxicity*
  • Hepatocytes / drug effects*
  • Hepatocytes / metabolism
  • Mice
  • Mice, Inbred C57BL
  • Oxidation-Reduction
  • Oxidative Stress / drug effects*
  • Oxidative Stress / genetics
  • Primary Cell Culture
  • Protein Structure, Secondary
  • Reactive Oxygen Species / metabolism

Substances

  • Decanoic Acids
  • Environmental Pollutants
  • Fluorocarbons
  • Reactive Oxygen Species
  • perfluorodecanoic acid
  • DNA
  • calf thymus DNA
  • Catalase