Injected laquinimod D-α-tocopheryl polyethylene glycol-1000 succinate polymeric micelles for the treatment of inflammatory bowel disease

Colloids Surf B Biointerfaces. 2020 Jan 1:185:110575. doi: 10.1016/j.colsurfb.2019.110575. Epub 2019 Oct 19.

Abstract

Inflammatory bowel diseases (IBDs) are chronic relapsing disorders of the gastrointestinal tract characterized pathologically by intestinal inflammation and epithelial injury. Laquinimod (LAQ), a poorly water-soluble compound, was proved to be effective for colitis remission at low dose of 0.5 mg/kg in patients with Crohn's disease. Due to its extremely low solubility in water, it was difficult to develop an injectable liquid dosage form. Herein, D-α-Tocopheryl polyethylene glycol-1000 succinate (TPGS) polymeric micelles were developed as a delivery vehicle of LAQ for the management of inflammatory bowel disease. Using the LAQ/TPGS ratio of 1:100, LAQ-loaded micelles were successfully prepared by thin-film dispersion method. The solubility of LAQ in water was significantly increased from 10.5 μg/mL in pure water to 500 μg/mL in TPGS micelles. LAQ-loaded micelles of TPGS exhibited the fine particle size of 34.6 nm and Zeta potential of -0.67 mV. Moreover, the good stability of LAQ-loaded micelles in physiology-mimicking medium was confirmed by detecting their particle size, zeta potential and leakage of the loading drug. Therapeutic effect of LAQ-loaded micelles on DSS-induced mice was proved by detecting DAI score, colon length and loss of body weight. Moreover, the morphology and colonic mucosal barrier of the injured colon of DSS-induced mice was largely recovered after treatment with LAQ-loaded micelles. Meanwhile, the inflammation of colitis colon was also obviously alleviated by LAQ-loaded micelles. Conclusively, polymeric micelles of TPGS may be a promising delivery vehicle of LAQ for the management of inflammatory bowel disease.

Keywords: Inflammatory bowel diseases; Injection; Laquinimod; Micelles; TPGS.

MeSH terms

  • Animals
  • Colon / drug effects
  • Colon / pathology
  • Dextran Sulfate
  • Drug Liberation
  • Inflammation / pathology
  • Inflammatory Bowel Diseases / drug therapy*
  • Inflammatory Bowel Diseases / pathology
  • Injections*
  • Intestinal Mucosa / drug effects
  • Intestinal Mucosa / pathology
  • Mice, Inbred ICR
  • Micelles*
  • Particle Size
  • Quinolones / pharmacology
  • Quinolones / therapeutic use*
  • Solubility
  • Spectroscopy, Fourier Transform Infrared
  • Static Electricity
  • Vitamin E / pharmacology
  • Vitamin E / therapeutic use*

Substances

  • Micelles
  • Quinolones
  • Vitamin E
  • Dextran Sulfate
  • laquinimod
  • tocophersolan