Ultrabright fluorescent silica nanoparticles for in vivo targeting of xenografted human tumors and cancer cells in zebrafish

Nanoscale. 2019 Nov 28;11(46):22316-22327. doi: 10.1039/c9nr06371d.

Abstract

New ultrabright fluorescent silica nanoparticles capable of the fast targeting of epithelial tumors in vivo are presented. The as-synthesized folate-functionalized ultrabright particles of 30-40 nm are 230 times brighter than quantum dots (QD450) and 50% brighter than the polymer dots with similar spectra (excitation 365 nm and emission 486 nm). To decrease non-specific targeting, particles are coated with polyethylene glycol (PEG). We demonstrate the in vivo targeting of xenographic human cervical epithelial tumors (HeLa cells) using zebrafish as a model system. The particles target tumors (and probably even individual HeLa cells) as small as 10-20 microns within 20-30 minutes after blood injection. To demonstrate the advantages of ultrabrightness, we repeated the experiments with similar but 200× less bright particles. Compared to those, ultrabright particles showed ∼3× faster tumor detection and ∼2× higher relative fluorescent contrast of tumors/cancer cells.

MeSH terms

  • Animals
  • Female
  • Folic Acid / chemistry
  • HeLa Cells
  • Humans
  • Nanoparticles / chemistry*
  • Neoplasms / diagnostic imaging*
  • Optical Imaging
  • Particle Size
  • Polyethylene Glycols / chemistry
  • Porosity
  • Silicon Dioxide / chemistry*
  • Transplantation, Heterologous
  • Zebrafish

Substances

  • Polyethylene Glycols
  • Silicon Dioxide
  • Folic Acid