8-Hydroxyquinoline-5-sulfonamides are promising antifungal candidates for the topical treatment of dermatomycosis

J Appl Microbiol. 2020 Apr;128(4):1038-1049. doi: 10.1111/jam.14545. Epub 2019 Dec 20.

Abstract

Aim: The purpose of this study was to uncover insights into the mechanism of action of the 8-hydroxyquinoline derivatives PH151 and PH153. In addition, with the future perspective of developing a topical drug for the treatment of candidiasis and dermatophytosis, the antifungal activity of a nanoemulsion formulation containing the most active compound (PH151) is also presented here.

Methods and results: Sorbitol protection assay and scanning electron microscopy indicate that the 8-hydroxyquinoline derivatives act on the cell wall of Candida sp. and dermatophytes and they inhibit the pseudohyphae formation of C. albicans. These findings demonstrate a strong effect of these compounds on C. albicans morphogenesis, which can be considered a potential mode of action for this molecule. Besides, the nanoemulsion formulation MIC values ranged from 0·5 to 4 μg ml-1 demonstrating the significant antifungal activity when incorporated into a pharmaceutical formulation.

Conclusions: Taken together, the results support the potential of these molecules as promising antifungal candidates for the treatment of candidiasis and dermatophytosis.

Significance and impact of the study: There is an emerging need to fill the pipeline with new antifungal drugs due to the limitations presented by the currently used drugs. In this study, we have described a novel formulation with a 8-hydroxyquinoline-5-sulfonamide derivative which has presented a great potency in providing a finished product. Furthermore, the derivative has shown a selective mechanism of action confirming its potential to be developed into a new drug candidate.

Keywords: antimicrobials; fungi; infection; mechanism of action; pharmaceuticals; pseudohyphae.

MeSH terms

  • Antifungal Agents / chemistry
  • Antifungal Agents / pharmacology*
  • Arthrodermataceae / drug effects*
  • Arthrodermataceae / growth & development
  • Candida albicans / drug effects
  • Candida albicans / growth & development
  • Candidiasis / drug therapy
  • Candidiasis / microbiology
  • Cell Wall / drug effects
  • Dermatomycoses / drug therapy
  • Dermatomycoses / microbiology*
  • Hyphae / drug effects
  • Hyphae / growth & development
  • Microbial Sensitivity Tests
  • Oxyquinoline / chemistry
  • Oxyquinoline / pharmacology*
  • Sulfonamides / chemistry
  • Sulfonamides / pharmacology*

Substances

  • Antifungal Agents
  • Sulfonamides
  • Oxyquinoline